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Title:Microfluidic control over topological states in channel-confined nematic flows
Authors:ID Čopar, Simon (Author)
ID Kos, Žiga (Author)
ID Emeršič, Tadej (Author)
ID Tkalec, Uroš (Author)
Files:.pdf Copar-2020-Microfluidic_control_over_topologic.pdf (7,79 MB)
MD5: 63400E45FE05ACB87484108B5CEBBCB7
 
URL https://doi.org/10.1038/s41467-019-13789-9
 
Language:English
Work type:Scientific work
Typology:1.01 - Original Scientific Article
Organization:FNM - Faculty of Natural Sciences and Mathematics
Abstract:Compared to isotropic liquids, orientational order of nematic liquid crystals makes their rheological properties more involved, and thus requires fine control of the flow parameters to govern the orientational patterns. In microfluidic channels with perpendicular surface alignment, nematics discontinuously transition from perpendicular structure at low flow rates to flow-aligned structure at high flow rates. Here we show how precise tuning of the driving pressure can be used to stabilize and manipulate a previously unresearched topologically protected chiral intermediate state which arises before the homeotropic to flow-aligned transition. We characterize the mechanisms underlying the transition and construct a phenomenological model to describe the critical behaviour and the phase diagram of the observed chiral flow state, and evaluate the effect of a forced symmetry breaking by introduction of a chiral dopant. Finally, we induce transitions on demand through channel geometry, application of laser tweezers, and careful control of the flow rate.
Keywords:nematic liquid crystals, microfluidics, topological states, nematic flows
Publication status:Published
Publication version:Version of Record
Submitted for review:28.07.2019
Article acceptance date:28.11.2019
Publication date:02.01.2020
Publisher:Nature Publishing Group
Year of publishing:2020
Number of pages:Str. 1-10
Numbering:Letn. 11, št. članka 59
PID:20.500.12556/DKUM-91564 New window
UDC:532.5
ISSN on article:2041-1723
COBISS.SI-ID:3400804 New window
DOI:10.1038/s41467-019-13789-9 New window
Publication date in DKUM:15.01.2025
Views:171
Downloads:14
Metadata:XML DC-XML DC-RDF
Categories:Misc.
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Record is a part of a journal

Title:Nature communications
Shortened title:Nat. Commun.
Publisher:Nature Publishing Group
ISSN:2041-1723
COBISS.SI-ID:2315876 New window

Document is financed by a project

Funder:ARRS - Slovenian Research Agency
Project number:P1-0099
Name:Fizika mehkih snovi, površin in nanostruktur

Funder:ARRS - Slovenian Research Agency
Project number:P1-0055
Name:Biofizika polimerov, membran, gelov, koloidov in celic

Funder:ARRS - Slovenian Research Agency
Project number:L1-8135
Name:Biološka zdravila: detektor tvorbe proteinskih delcev na osnovi tekočih kristalov

Funder:ARRS - Slovenian Research Agency
Project number:J1-9149
Name:Orientacijske interakcije v posplošenem Thomsonovem problemu: dipolna stabilizacija sferičnih nanostruktur

Funder:ARRS - Slovenian Research Agency
Project number:N1-0124
Name:Geometrijsko in topološko vodenje aktivnih elastomerov

Funder:Other - Other funder or multiple funders
Project number:CA17139
Acronym:COST Action

Licences

License:CC BY 4.0, Creative Commons Attribution 4.0 International
Link:http://creativecommons.org/licenses/by/4.0/
Description:This is the standard Creative Commons license that gives others maximum freedom to do what they want with the work as long as they credit the author.
Licensing start date:02.01.2020

Secondary language

Language:Slovenian
Keywords:nematski tekoči kristali, mikrofluidika, topološka stanja, nematski tokovi


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